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4 Studies on stereoselective polymerization of racemic olefins also support this view 38 Polymerization of 3,7-dimethyl-I-octene (the chiral center is in CJ position to the double bond) took place with 90% stereoselectivity yielding an equimolar mixture of homopolymers of the two enantiomers No stereoselectivity was observed in the polymerization of 5-methyl-I-heptene (the chiral center is in y position to the double bond) The conclusion is that the ability of a catalytic center to distinguish between the two enantiomers of a monomer required for stereoselective polymerization must arise from its intrinsic asymmetry The first-ever chiral polypropylene synthesized using a chiral zirconium complex with aluminoxane cocatalyst is the latest evidence to testify the role of the catalyst center in isotactic polymerization 339 These observations clearly indicate that heterogeneous Ziegler-Natta catalysts must contain chiral active centers.

consists of the k-bit pre x determined by the contents of the leftmost k-stages concatenated with the output of a (N 2 k)-stage LFSR. Proposition 8.1: An N-stage LFSR with feedback coef cients (c0, c1, . . . , cN) enjoys the following properties: 8.1a If s(t) s(t), then s(t 1) s(t 1) and s(t 2 1) s(t 2 1); 8.1b If s(t) (0)N ; (0, 0, . . . , 0), the output remains null for t . t ; 8.1c The sequence of states s(0), s(1), . . . , s( P 2 1) are distinct and periodic with period P; s(0) s(P), with P satisfying 1 P 2N 2 1. Proof of (8.1a):

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It is conceivable to assume that the asymmetric ligand environment is responsible for the regio- and stereoselectivity of these systems Typical isospecific catalysts are the TiCl 3-based systems, both the first-generation heterogeneous Ziegler-Natta catalysts and the high-activity MgCITsupported catalysts 40 It also follows that the key factor in stereoregulation is the favored discriminative complexation at one of the prochiral faces of the olefin followed by stereospecific insertion Various models of catalytic centers and mechanisms have been proposed to interpret the origin of stereoregular polymerization 208 ,254,295,328,340 The Cossee-Arlman mechanism discussed before for ethylene polymerization 303 ,304 offers a conceivable explanation for stereoregulation 05,306 According to this model, alkylated hexacoordinated titanium atoms with one vacant octahedral site characteristic of CJ-, y-, and o-TiC1 3 serve as asymmetric catalytic sites (45) [see displayed structure preceding Eq (1365)].

Fadiman, Clifton Fantasia Mathemoiua New York: Simon and Schuster, 1958 (Stories, poetry, and other oddments) Galton, Francis Hereditary Genius: An Inquiry into Its Laws and Consequences New York: Horizon Press, 1952 (Orig pub 1869) (Some historical information about the Bernoulli brothers) Gillispie, Charles C, ed Dutionary cff &!entific Biography 16 vols New York: Scnbner, 1970-1980 Goldstein, Catharine, and Jeremy Gray "The Roots of Modern Maths (From the Middle Ages to the Enlightenment)," UNESCO Couna (November 1989): 42ff Grattan Guinness, Ivor The N()1'(on History cffthe MathemoJual SaenceJ New York: W W Norton, 1998 Guedj, Denis The Rurot's Theorem New York: St Martin's, 2000 (A combined mystery and quick tour of the history of mathematics) Guillen, Michael Five Equation> That Clumged the World: The Rrwer and RJetry cffMathematics New York: Hyperion, 1995 Gullberg,jan Mathematics: From the Birth cffNumhers New York: W W Norton, 1997 Hellman, Hal.

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